Trion fine structure and coupled spin-valley dynamics in monolayer tungsten disulfide View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-09-02

AUTHORS

Gerd Plechinger, Philipp Nagler, Ashish Arora, Robert Schmidt, Alexey Chernikov, Andrés Granados del Águila, Peter C.M. Christianen, Rudolf Bratschitsch, Christian Schüller, Tobias Korn

ABSTRACT

Monolayer transition-metal dichalcogenides have recently emerged as possible candidates for valleytronic applications, as the spin and valley pseudospin are directly coupled and stabilized by a large spin splitting. The optical properties of these two-dimensional crystals are dominated by tightly bound electron-hole pairs (excitons) and more complex quasiparticles such as charged excitons (trions). Here we investigate monolayer WS2 samples via photoluminescence and time-resolved Kerr rotation. In photoluminescence and in energy-dependent Kerr rotation measurements, we are able to resolve two different trion states, which we interpret as intravalley and intervalley trions. Using time-resolved Kerr rotation, we observe a rapid initial valley polarization decay for the A exciton and the trion states. Subsequently, we observe a crossover towards exciton-exciton interaction-related dynamics, consistent with the formation and decay of optically dark A excitons. By contrast, resonant excitation of the B exciton transition leads to a very slow decay of the Kerr signal. More... »

PAGES

12715

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms12715

DOI

http://dx.doi.org/10.1038/ncomms12715

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1051055301

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27586517


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