Unassisted photoelectrochemical water splitting exceeding 7% solar-to-hydrogen conversion efficiency using photon recycling View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-06-21

AUTHORS

Xinjian Shi, Hokyeong Jeong, Seung Jae Oh, Ming Ma, Kan Zhang, Jeong Kwon, In Taek Choi, Il Yong Choi, Hwan Kyu Kim, Jong Kyu Kim, Jong Hyeok Park

ABSTRACT

Various tandem cell configurations have been reported for highly efficient and spontaneous hydrogen production from photoelectrochemical solar water splitting. However, there is a contradiction between two main requirements of a front photoelectrode in a tandem cell configuration, namely, high transparency and high photocurrent density. Here we demonstrate a simple yet highly effective method to overcome this contradiction by incorporating a hybrid conductive distributed Bragg reflector on the back side of the transparent conducting substrate for the front photoelectrochemical electrode, which functions as both an optical filter and a conductive counter-electrode of the rear dye-sensitized solar cell. The hybrid conductive distributed Bragg reflectors were designed to be transparent to the long-wavelength part of the incident solar spectrum (λ>500 nm) for the rear solar cell, while reflecting the short-wavelength photons (λ<500 nm) which can then be absorbed by the front photoelectrochemical electrode for enhanced photocurrent generation. More... »

PAGES

11943

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms11943

DOI

http://dx.doi.org/10.1038/ncomms11943

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1027254038

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27324578


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