Freestanding three-dimensional core–shell nanoarrays for lithium-ion battery anodes View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-06-03

AUTHORS

Guoqiang Tan, Feng Wu, Yifei Yuan, Renjie Chen, Teng Zhao, Ying Yao, Ji Qian, Jianrui Liu, Yusheng Ye, Reza Shahbazian-Yassar, Jun Lu, Khalil Amine

ABSTRACT

Structural degradation and low conductivity of transition-metal oxides lead to severe capacity fading in lithium-ion batteries. Recent efforts to solve this issue have mainly focused on using nanocomposites or hybrids by integrating nanosized metal oxides with conducting additives. Here we design specific hierarchical structures and demonstrate their use in flexible, large-area anode assemblies. Fabrication of these anodes is achieved via oxidative growth of copper oxide nanowires onto copper substrates followed by radio-frequency sputtering of carbon-nitride films, forming freestanding three-dimensional arrays with core-shell nano-architecture. Cable-like copper oxide/carbon-nitride core-shell nanostructures accommodate the volume change during lithiation-delithiation processes, the three-dimensional arrays provide abundant electroactive zones and electron/ion transport paths, and the monolithic sandwich-type configuration without additional binders or conductive agents improves energy/power densities of the whole electrode. More... »

PAGES

11774

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms11774

DOI

http://dx.doi.org/10.1038/ncomms11774

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1002448053

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27256920


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