Intrinsic correlation between β-relaxation and spatial heterogeneity in a metallic glass View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-05-09

AUTHORS

F. Zhu, H. K. Nguyen, S. X. Song, Daisman P. B. Aji, A. Hirata, H. Wang, K. Nakajima, M. W. Chen

ABSTRACT

β-relaxation has long been attributed to localized motion of constituent molecules or atoms confined to isolated regions in glasses. However, direct experimental evidence to support this spatially heterogeneous scenario is still missing. Here we report the evolution of nanoscale structural heterogeneity in a metallic glass during β-relaxation by utilizing amplitude-modulation dynamic atomic force microscopy. The successive degeneration of heterogeneity during β-relaxation can be well described by the Kohlrausch–Williams–Watts equation. The characteristic relaxation time and activation energy of the heterogeneity evolution are in accord with those of excess enthalpy release by β-relaxation. Our study correlates β-relaxation with nanoscale spatial heterogeneity and provides direct evidence on the structural origins of β-relaxation in metallic glasses. More... »

PAGES

11516

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms11516

DOI

http://dx.doi.org/10.1038/ncomms11516

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1049615186

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27158084


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