Controllable positive exchange bias via redox-driven oxygen migration View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-03-21

AUTHORS

Dustin A. Gilbert, Justin Olamit, Randy K. Dumas, B. J. Kirby, Alexander J. Grutter, Brian B. Maranville, Elke Arenholz, Julie A. Borchers, Kai Liu

ABSTRACT

Ionic transport in metal/oxide heterostructures offers a highly effective means to tailor material properties via modification of the interfacial characteristics. However, direct observation of ionic motion under buried interfaces and demonstration of its correlation with physical properties has been challenging. Using the strong oxygen affinity of gadolinium, we design a model system of GdxFe1-x/NiCoO bilayer films, where the oxygen migration is observed and manifested in a controlled positive exchange bias over a relatively small cooling field range. The exchange bias characteristics are shown to be the result of an interfacial layer of elemental nickel and cobalt, a few nanometres in thickness, whose moments are larger than expected from uncompensated NiCoO moments. This interface layer is attributed to a redox-driven oxygen migration from NiCoO to the gadolinium, during growth or soon after. These results demonstrate an effective path to tailoring the interfacial characteristics and interlayer exchange coupling in metal/oxide heterostructures. More... »

PAGES

11050

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms11050

DOI

http://dx.doi.org/10.1038/ncomms11050

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1009043486

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26996674


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274 rdf:type schema:Organization
275 https://www.grid.ac/institutes/grid.8761.8 schema:alternateName University of Gothenburg
276 schema:name Department of Physics, University of Gothenburg, Gothenburg 412 96, Sweden
277 Physics Department, University of California, Davis, One Shields Avenue, Davis, California 95616, USA
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279 https://www.grid.ac/institutes/grid.94225.38 schema:alternateName National Institute of Standards and Technology
280 schema:name NIST Center for Neutron Research, Gaithersburg, Maryland 20899, USA
281 Physics Department, University of California, Davis, One Shields Avenue, Davis, California 95616, USA
282 rdf:type schema:Organization
 




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