Pure and stable metallic phase molybdenum disulfide nanosheets for hydrogen evolution reaction View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-02-10

AUTHORS

Xiumei Geng, Weiwei Sun, Wei Wu, Benjamin Chen, Alaa Al-Hilo, Mourad Benamara, Hongli Zhu, Fumiya Watanabe, Jingbiao Cui, Tar-pin Chen

ABSTRACT

Metallic-phase MoS2 (M-MoS2) is metastable and does not exist in nature. Pure and stable M-MoS2 has not been previously prepared by chemical synthesis, to the best of our knowledge. Here we report a hydrothermal process for synthesizing stable two-dimensional M-MoS2 nanosheets in water. The metal-metal Raman stretching mode at 146 cm(-1) in the M-MoS2 structure, as predicted by theoretical calculations, is experimentally observed. The stability of the M-MoS2 is associated with the adsorption of a monolayer of water molecules on both sides of the nanosheets, which reduce restacking and prevent aggregation in water. The obtained M-MoS2 exhibits excellent stability in water and superior activity for the hydrogen evolution reaction, with a current density of 10 mA cm(-2) at a low potential of -175 mV and a Tafel slope of 41 mV per decade. More... »

PAGES

10672

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms10672

DOI

http://dx.doi.org/10.1038/ncomms10672

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1020677392

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26861766


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37 schema:description Metallic-phase MoS2 (M-MoS2) is metastable and does not exist in nature. Pure and stable M-MoS2 has not been previously prepared by chemical synthesis, to the best of our knowledge. Here we report a hydrothermal process for synthesizing stable two-dimensional M-MoS2 nanosheets in water. The metal-metal Raman stretching mode at 146 cm(-1) in the M-MoS2 structure, as predicted by theoretical calculations, is experimentally observed. The stability of the M-MoS2 is associated with the adsorption of a monolayer of water molecules on both sides of the nanosheets, which reduce restacking and prevent aggregation in water. The obtained M-MoS2 exhibits excellent stability in water and superior activity for the hydrogen evolution reaction, with a current density of 10 mA cm(-2) at a low potential of -175 mV and a Tafel slope of 41 mV per decade.
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