Three-dimensional porous carbon composites containing high sulfur nanoparticle content for high-performance lithium–sulfur batteries View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-02-01

AUTHORS

Guoxing Li, Jinhua Sun, Wenpeng Hou, Shidong Jiang, Yong Huang, Jianxin Geng

ABSTRACT

Sulfur is a promising cathode material for lithium-sulfur batteries because of its high theoretical capacity (1,675 mA h g(-1)); however, its low electrical conductivity and the instability of sulfur-based electrodes limit its practical application. Here we report a facile in situ method for preparing three-dimensional porous graphitic carbon composites containing sulfur nanoparticles (3D S@PGC). With this strategy, the sulfur content of the composites can be tuned to a high level (up to 90 wt%). Because of the high sulfur content, the nanoscale distribution of the sulfur particles, and the covalent bonding between the sulfur and the PGC, the developed 3D S@PGC cathodes exhibit excellent performance, with a high sulfur utilization, high specific capacity (1,382, 1,242 and 1,115 mA h g(-1) at 0.5, 1 and 2 C, respectively), long cycling life (small capacity decay of 0.039% per cycle over 1,000 cycles at 2 C) and excellent rate capability at a high charge/discharge current. More... »

PAGES

10601

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms10601

DOI

http://dx.doi.org/10.1038/ncomms10601

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1050622004

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26830732


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