A pervasive role for biomass burning in tropical high ozone/low water structures View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2016-01-13

AUTHORS

Daniel C. Anderson, Julie M. Nicely, Ross J. Salawitch, Timothy P. Canty, Russell R. Dickerson, Thomas F. Hanisco, Glenn M. Wolfe, Eric C. Apel, Elliot Atlas, Thomas Bannan, Stephane Bauguitte, Nicola J. Blake, James F. Bresch, Teresa L. Campos, Lucy J. Carpenter, Mark D. Cohen, Mathew Evans, Rafael P. Fernandez, Brian H. Kahn, Douglas E. Kinnison, Samuel R. Hall, Neil R.P. Harris, Rebecca S. Hornbrook, Jean-Francois Lamarque, Michael Le Breton, James D. Lee, Carl Percival, Leonhard Pfister, R. Bradley Pierce, Daniel D. Riemer, Alfonso Saiz-Lopez, Barbara J.B. Stunder, Anne M. Thompson, Kirk Ullmann, Adam Vaughan, Andrew J. Weinheimer

ABSTRACT

Air parcels with mixing ratios of high O3 and low H2O (HOLW) are common features in the tropical western Pacific (TWP) mid-troposphere (300-700 hPa). Here, using data collected during aircraft sampling of the TWP in winter 2014, we find strong, positive correlations of O3 with multiple biomass burning tracers in these HOLW structures. Ozone levels in these structures are about a factor of three larger than background. Models, satellite data and aircraft observations are used to show fires in tropical Africa and Southeast Asia are the dominant source of high O3 and that low H2O results from large-scale descent within the tropical troposphere. Previous explanations that attribute HOLW structures to transport from the stratosphere or mid-latitude troposphere are inconsistent with our observations. This study suggest a larger role for biomass burning in the radiative forcing of climate in the remote TWP than is commonly appreciated. More... »

PAGES

10267

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms10267

DOI

http://dx.doi.org/10.1038/ncomms10267

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1044067194

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26758808


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75 schema:description Air parcels with mixing ratios of high O3 and low H2O (HOLW) are common features in the tropical western Pacific (TWP) mid-troposphere (300-700 hPa). Here, using data collected during aircraft sampling of the TWP in winter 2014, we find strong, positive correlations of O3 with multiple biomass burning tracers in these HOLW structures. Ozone levels in these structures are about a factor of three larger than background. Models, satellite data and aircraft observations are used to show fires in tropical Africa and Southeast Asia are the dominant source of high O3 and that low H2O results from large-scale descent within the tropical troposphere. Previous explanations that attribute HOLW structures to transport from the stratosphere or mid-latitude troposphere are inconsistent with our observations. This study suggest a larger role for biomass burning in the radiative forcing of climate in the remote TWP than is commonly appreciated.
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