Enhancing the magnetic anisotropy of maghemite nanoparticles via the surface coordination of molecular complexes View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2015-12

AUTHORS

Yoann Prado, Niéli Daffé, Aude Michel, Thomas Georgelin, Nader Yaacoub, Jean-Marc Grenèche, Fadi Choueikani, Edwige Otero, Philippe Ohresser, Marie-Anne Arrio, Christophe Cartier-dit-Moulin, Philippe Sainctavit, Benoit Fleury, Vincent Dupuis, Laurent Lisnard, Jérôme Fresnais

ABSTRACT

Superparamagnetic nanoparticles are promising objects for data storage or medical applications. In the smallest--and more attractive--systems, the properties are governed by the magnetic anisotropy. Here we report a molecule-based synthetic strategy to enhance this anisotropy in sub-10-nm nanoparticles. It consists of the fabrication of composite materials where anisotropic molecular complexes are coordinated to the surface of the nanoparticles. Reacting 5 nm γ-Fe2O3 nanoparticles with the [Co(II)(TPMA)Cl2] complex (TPMA: tris(2-pyridylmethyl)amine) leads to the desired composite materials and the characterization of the functionalized nanoparticles evidences the successful coordination--without nanoparticle aggregation and without complex dissociation--of the molecular complexes to the nanoparticles surface. Magnetic measurements indicate the significant enhancement of the anisotropy in the final objects. Indeed, the functionalized nanoparticles show a threefold increase of the blocking temperature and a coercive field increased by one order of magnitude. More... »

PAGES

10139

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/ncomms10139

DOI

http://dx.doi.org/10.1038/ncomms10139

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1031732063

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26634987


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