Molecular understanding of sulphuric acid–amine particle nucleation in the atmosphere View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2013-10

AUTHORS

João Almeida, Siegfried Schobesberger, Andreas Kürten, Ismael K. Ortega, Oona Kupiainen-Määttä, Arnaud P. Praplan, Alexey Adamov, Antonio Amorim, Federico Bianchi, Martin Breitenlechner, André David, Josef Dommen, Neil M. Donahue, Andrew Downard, Eimear Dunne, Jonathan Duplissy, Sebastian Ehrhart, Richard C. Flagan, Alessandro Franchin, Roberto Guida, Jani Hakala, Armin Hansel, Martin Heinritzi, Henning Henschel, Tuija Jokinen, Heikki Junninen, Maija Kajos, Juha Kangasluoma, Helmi Keskinen, Agnieszka Kupc, Theo Kurtén, Alexander N. Kvashin, Ari Laaksonen, Katrianne Lehtipalo, Markus Leiminger, Johannes Leppä, Ville Loukonen, Vladimir Makhmutov, Serge Mathot, Matthew J. McGrath, Tuomo Nieminen, Tinja Olenius, Antti Onnela, Tuukka Petäjä, Francesco Riccobono, Ilona Riipinen, Matti Rissanen, Linda Rondo, Taina Ruuskanen, Filipe D. Santos, Nina Sarnela, Simon Schallhart, Ralf Schnitzhofer, John H. Seinfeld, Mario Simon, Mikko Sipilä, Yuri Stozhkov, Frank Stratmann, Antonio Tomé, Jasmin Tröstl, Georgios Tsagkogeorgas, Petri Vaattovaara, Yrjo Viisanen, Annele Virtanen, Aron Vrtala, Paul E. Wagner, Ernest Weingartner, Heike Wex, Christina Williamson, Daniela Wimmer, Penglin Ye, Taina Yli-Juuti, Kenneth S. Carslaw, Markku Kulmala, Joachim Curtius, Urs Baltensperger, Douglas R. Worsnop, Hanna Vehkamäki, Jasper Kirkby

ABSTRACT

Nucleation of aerosol particles from trace atmospheric vapours is thought to provide up to half of global cloud condensation nuclei. Aerosols can cause a net cooling of climate by scattering sunlight and by leading to smaller but more numerous cloud droplets, which makes clouds brighter and extends their lifetimes. Atmospheric aerosols derived from human activities are thought to have compensated for a large fraction of the warming caused by greenhouse gases. However, despite its importance for climate, atmospheric nucleation is poorly understood. Recently, it has been shown that sulphuric acid and ammonia cannot explain particle formation rates observed in the lower atmosphere. It is thought that amines may enhance nucleation, but until now there has been no direct evidence for amine ternary nucleation under atmospheric conditions. Here we use the CLOUD (Cosmics Leaving OUtdoor Droplets) chamber at CERN and find that dimethylamine above three parts per trillion by volume can enhance particle formation rates more than 1,000-fold compared with ammonia, sufficient to account for the particle formation rates observed in the atmosphere. Molecular analysis of the clusters reveals that the faster nucleation is explained by a base-stabilization mechanism involving acid-amine pairs, which strongly decrease evaporation. The ion-induced contribution is generally small, reflecting the high stability of sulphuric acid-dimethylamine clusters and indicating that galactic cosmic rays exert only a small influence on their formation, except at low overall formation rates. Our experimental measurements are well reproduced by a dynamical model based on quantum chemical calculations of binding energies of molecular clusters, without any fitted parameters. These results show that, in regions of the atmosphere near amine sources, both amines and sulphur dioxide should be considered when assessing the impact of anthropogenic activities on particle formation. More... »

PAGES

359

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/nature12663

DOI

http://dx.doi.org/10.1038/nature12663

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1002282333

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/24097350


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