Loss of superconductivity with the addition of Al to MgB2 and a structural transition in Mg1-x AlxB2 View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2001-03

AUTHORS

J. S. Slusky, N. Rogado, K. A. Regan, M. A. Hayward, P. Khalifah, T. He, K. Inumaru, S. M. Loureiro, M. K. Haas, H. W. Zandbergen, R. J. Cava

ABSTRACT

The basic magnetic and electronic properties of most binary compounds have been well known for decades. The recent discovery of superconductivity at 39 K in the simple binary ceramic compound magnesium diboride, MgB2, was therefore surprising. Indeed, this material has been known and structurally characterized since the mid 1950s (ref. 2), and is readily available from chemical suppliers (it is commonly used as a starting material for chemical metathesis reactions). Here we show that the addition of electrons to MgB2, through partial substitution of Al for Mg, results in the loss of superconductivity. Associated with the Al substitution is a subtle but distinct structural transition, reflected in the partial collapse of the spacing between boron layers near an Al content of 10 per cent. This indicates that superconducting MgB2 is poised very near a structural instability at slightly higher electron concentrations. More... »

PAGES

343

References to SciGraph publications

Journal

TITLE

Nature

ISSUE

6826

VOLUME

410

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1038/35066528

DOI

http://dx.doi.org/10.1038/35066528

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1000232825

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/11268204


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