The Experimental Nuclear Quadrupole Interaction in Synthetic Al-Goethites of Varying Crystallinity View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2003-06

AUTHORS

C. A. Barrero, R. E. Vandenberghe, E. De Grave, A. L. Morales, G. Pérez

ABSTRACT

The effect of aluminum content and degree of crystallinity upon the possible values for both the polar coordinates (Θ and ϕ) of the magnetic hyperfine field direction with respect to the electric field gradient (EFG) frame of reference and for the asymmetry parameter (η) in synthetic Al-goethites was determined experimentally from their variable temperature Mössbauer spectra. The range of values for these parameters was examined using the ratio R of the quadrupole shift to the quadrupole splitting. It was found that R varies in the range −0.62≤R≤−0.55, implying that, considering all the samples, ∼65°≤Θ≤90°, ∼−1≤cos 2ϕ≤−0.25 and ∼0.1≤η≤1. Additionally, the principal components of the EFG tensor and η were calculated using the simple point charge model. More... »

PAGES

337-344

Journal

TITLE

Hyperfine Interactions

ISSUE

1-4

VOLUME

148-149

Identifiers

URI

http://scigraph.springernature.com/pub.10.1023/b:hype.0000003796.91461.8a

DOI

http://dx.doi.org/10.1023/b:hype.0000003796.91461.8a

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1007455742


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