Isotopic Study of N2O Decomposition on an Ion-Exchanged Fe-Zeolite Catalyst: Mechanism of O2 Formation View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2002-10

AUTHORS

Takeshi Nobukawa, Shin-ichi Tanaka, Shin-ichi Ito, Keiichi Tomishige, Satoshi Kameoka, Kimio Kunimori

ABSTRACT

N2O decomposition on an ion-exchanged Fe-MFI catalyst has been studied using an 18O-tracer technique in order to reveal the reaction mechanism. N216O was pulsed onto an 18O2-treated Fe-MFI catalyst at 693 K, and the O2 molecules produced were monitored by means of mass spectrometry. The 18O fraction in the produced oxygen had almost half the value of that on the surface oxygen, and 18O18O was not detected. The result shows that O2 formation proceeds via the Eley–Rideal mechanism (N216O + 18O(a) → N2 + 16O18O). More... »

PAGES

5-8

Journal

TITLE

Catalysis Letters

ISSUE

1-2

VOLUME

83

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1023/a:1020636910973

DOI

http://dx.doi.org/10.1023/a:1020636910973

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1051111308


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