Effect of support on the conversion of methane to synthesis gas over supported iridium catalysts View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

1998-05

AUTHORS

Kiyoharu Nakagawa, Kengo Anzai, Naoko Matsui, Naoki Ikenaga, Toshimitsu Suzuki, Yonghong Teng, Tetsuhiko Kobayashi, Masatake Haruta

ABSTRACT

A partial oxidation of methane was carried out using iridium catalysts supported on several metal oxides. The productivity of the synthesis gas from methane was strongly affected by the choice of support oxides for the catalysts. The synthesis gas production proceeded basically via a two-step reaction consisting of methane combustion to give H2O and CO2, followed by the reforming of methane from CO2 and steam. Although the combustion and the reforming of methane from steam did not depend upon the catalyst support, a large variation in the catalytic activity for the reforming of methane from CO2 was observed over Ir catalysts with different supports. The support activity order in the reforming of methane from CO2 with iridium catalysts was as follows: TiO2≧ZrO2≧Y2O3>La2O3>MgO≧Al2O3>SiO2. The same order was observed in the synthesis gas production from the partial oxidation of methane. More... »

PAGES

163-167

Journal

TITLE

Catalysis Letters

ISSUE

3-4

VOLUME

51

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1023/a:1019065824331

DOI

http://dx.doi.org/10.1023/a:1019065824331

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1031469655


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