Making gold less noble View Full Text


Ontology type: schema:ScholarlyArticle      Open Access: True


Article Info

DATE

2000-02

AUTHORS

M. Mavrikakis, P. Stoltze, J.K. Nørskov

ABSTRACT

Self‐consistent density functional calculations for the adsorption of O and CO on flat and stepped Au(111) surfaces are used to investigate effects which may increase the reactivity of Au. We find that the adsorption energy does not depend on the number of Au layers if there are more than two layers. Steps are found to bind considerably stronger than the (111) terraces, and an expansive strain has the same effect. On this basis we suggest that the unusually large catalytic activity of highly‐dispersed Au particles may in part be due to high step densities on the small particles and/or strain effects due to the mismatch at the Au–support interface. More... »

PAGES

101-106

Identifiers

URI

http://scigraph.springernature.com/pub.10.1023/a:1019028229377

DOI

http://dx.doi.org/10.1023/a:1019028229377

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1043166310


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