The role of Cu crystallographic orientations towards growing superclean graphene on meter-sized scale View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2021-11-04

AUTHORS

Xiaoting Liu, Jincan Zhang, Wendong Wang, Wei Zhao, Heng Chen, Bingyao Liu, Mengqi Zhang, Fushun Liang, Lijuan Zhang, Rui Zhang, Ning Li, Yuexin Zhang, Yuchen Liu, Kaicheng Jia, Luzhao Sun, Yixuan Zhao, Peng Gao, Qinghong Yuan, Li Lin, Hailin Peng, Zhongfan Liu

ABSTRACT

Chemical vapor deposition (CVD)-grown graphene films on Cu foils, exhibiting fine scalability and high quality, are still suffering from the adverse impact of surface contamination, i.e., amorphous carbon. Despite the recent successful preparation of superclean graphene through Cu-vapor-assisted reactions, the formation mechanism of amorphous carbon remains unclear, especially with regard to the functions of substrates. Herein, we have found that the crystallographic orientations of underlying metal substrates would determine the cleanness of graphene in such a way that slower diffusion of active carbon species on as-formed graphene-Cu(100) surface is the key factor that suppresses the formation of contamination. The facile synthesis of clean graphene is achieved on the meter-sized Cu(100) that is transformed from the polycrystalline Cu foils. Furthermore, a clean surface of graphene on Cu(100) ensures the reduction of transfer-related polymer residues, and enhanced optical and electrical performance, which allows for versatile applications of graphene in biosensors, functioning as flexible transparent electrodes. This work would offer a promising material platform for the fundamental investigation and create new opportunities for the advanced applications of high-quality graphene films. More... »

PAGES

3775-3780

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s12274-021-3922-x

DOI

http://dx.doi.org/10.1007/s12274-021-3922-x

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1142400922


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