One-step synthesis of magnetically recyclable Au/Co/Fe triple-layered core-shell nanoparticles as highly efficient catalysts for the hydrolytic dehydrogenation of ammonia borane View Full Text


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Article Info

DATE

2011-12

AUTHORS

Kengo Aranishi, Hai-Long Jiang, Tomoki Akita, Masatake Haruta, Qiang Xu

ABSTRACT

Magnetically recyclable Au/Co/Fe core-shell nanoparticles (NPs) have been successfully synthesized via a one-step in situ procedure. Transmission electron microscope (TEM), energy dispersive X-ray spectroscopic (EDS), and electron energy-loss spectroscopic (EELS) measurements revealed that the trimetallic Au/Co/Fe NPs have a triple-layered core-shell structure composed of a Au core, a Co-rich inter-layer, and a Fe-rich shell. The Au/Co/Fe core-shell NPs exhibit much higher catalytic activities for hydrolytic dehydrogenation of ammonia borane (NH3BH3, AB) than the monometallic (Au, Co, Fe) or bimetallic (AuCo, AuFe, CoFe) counterparts. More... »

PAGES

1233-1241

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s12274-011-0174-1

DOI

http://dx.doi.org/10.1007/s12274-011-0174-1

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1051771881


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