Synthesis of Tb3+ ion doped ZnWO4 phosphors and investigation of their photoluminescence properties: concentration effect View Full Text


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Article Info

DATE

2019-06

AUTHORS

N Premjit Singh, Y Rangeela Devi, N Rajmuhon Singh, N Mohondas Singh

ABSTRACT

In this paper, the effects of Tb3+ ion concentration on the structural and photoluminescence properties of ZnWO4:Tb3+ have been reported. X-ray diffraction studies indicated that the monoclinic structure of the samples and the crystallinity were found to decrease with the increase of Tb3+ ion concentration due to the distortion in the crystal lattice. The formation of the monoclinic structure was further supported by high resolution transmission electron microscopy and Fourier transform infrared analyses. The transmission electron microscopy image of ZnWO4:Tb3+ (7%) showed a spherical morphology with crystallite sizes in the range of ∼8–12 nm. The excitation spectrum showed a strong broad band originated from the electronic transition within the WO66- group. Upon excitation at 270 nm, the prepared ZnWO4:Tb3+ phosphors exhibited sharp and narrow emission peaks, characteristic of the f–f transitions of Tb3+ ions besides a broad band with the maximum at around 460 nm due to the host lattice. The intensity of the broad emission band was found to decrease gradually with the increase of Tb3+ ion concentration and reached minimum at 7 at%. The decay time of the prepared phosphors was investigated in detail and the maximum average lifetime value is found to be 1.187 ms. More... »

PAGES

96

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http://scigraph.springernature.com/pub.10.1007/s12034-019-1794-4

DOI

http://dx.doi.org/10.1007/s12034-019-1794-4

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