Tamarind shell tannin-doped hybrid sol–gel coatings on mild steel in acidic medium toward improved corrosion protection View Full Text


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Article Info

DATE

2021-11-09

AUTHORS

Abdullahi Abdulmajid, Tuan Sherwyn Hamidon, M. Hazwan Hussin

ABSTRACT

This study investigated the application of tamarind shell tannin extracts (TSTE) [isolated using methanol (TME) and 70% acetone (TAE)]-doped hybrid sol–gel coatings prepared using (3-Glycidyloxypropyl)trimethoxysilane (GPTMS) and tetraethoxysilane (TEOS) in 0.5 M HCl solution. The anticorrosion properties of these hybrid coatings on the surface of mild steel electrodes were described using potentiodynamic polarization (PD) and electrochemical impedance spectroscopy (EIS) measurements. The hybrid sol–gel coatings were characterized via FTIR. Also, the hydrophobicity of the coated plates was determined through water contact angle measurement. Meanwhile, the surface morphology and elemental compositions were determined using SEM/EDX analyses. The electrochemical measurements showed that the mixture of doped TME and TAE hybrid sol–gel coating resulted in higher corrosion resistance. The corrosion inhibition efficiency (CE) was CETME = 94.02% and CETAE = 91.35%, respectively. The Tafel slopes revealed a mixed form of corrosion protection with the main effect at cathodic sites. FTIR absorption bands attained at 945 cm−1 for TME and 961 cm−1 for TAE revealed Fe–O–Si bond formation. The higher corrosion inhibition capability of the coating matrix corroborates to higher water contact angle (θTME = 107.64°, θTAE = 104.62°) values. SEM analysis revealed coatings' improved corrosion protection due to the doping's enhanced inhibitive performance. More... »

PAGES

527-542

References to SciGraph publications

  • 2020-06-30. Extracts of curcumin-incorporated hybrid sol–gel coatings for the corrosion mitigation of mild steel in 0.5 M HCl in JOURNAL OF COATINGS TECHNOLOGY AND RESEARCH
  • 2012-02-28. “Quebracho” tannin derivative and boosters biocides for new antifouling formulations in JOURNAL OF COATINGS TECHNOLOGY AND RESEARCH
  • 2021-01-29. Enhanced corrosion inhibition of low carbon steel in aqueous sodium chloride employing sol–gel-based hybrid silanol coatings in JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY
  • 2007-05-08. Synthesis and characterization of sol–gel derived glass-ceramic and its corrosion protection on 316L SS in JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY
  • 1992. Complexation of Condensed Tannins with Metal Ions in PLANT POLYPHENOLS
  • 2015-02-13. Effect of the addition of 3-glycidoxypropyltrimethoxysilane to tetraethoxyorthosilicate-based stone protective coating using n-octylamine as a catalyst in BULLETIN OF MATERIALS SCIENCE
  • 2010-02-25. Inorganic–organic sol gel hybrid coatings for corrosion protection of metals in JOURNAL OF SOL-GEL SCIENCE AND TECHNOLOGY
  • 2014-07. Corrosion performance of rosemary-extract-doped TEOS:TMSM sol-gel coatings on 304L stainless steel in SURFACE ENGINEERING AND APPLIED ELECTROCHEMISTRY
  • 2012-03-14. Features of the occurrence of electrochemical processes in contact of sodium chloride solutions with the surface of superhydrophobic coatings on titanium in RUSSIAN JOURNAL OF ELECTROCHEMISTRY
  • 2006-11-28. Study of the hydrolysis and condensation of γ-Aminopropyltriethoxysilane by FT-IR spectroscopy in JOURNAL OF MATERIALS SCIENCE
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    http://scigraph.springernature.com/pub.10.1007/s11998-021-00539-0

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