Enhanced visible-light-driven photocatalysis of Bi2YO4Cl heterostructures functionallized by bimetallic RhNi nanoparticles View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-12

AUTHORS

Palepu Teja Ravindar, Vidya Sagar Choppella, Anil Kumar Mokshagundam, M. Kiruba, Sunil G. Babu, Korupolu Raghu Babu, L. John Berchmans, Gosipathala Sreedhar

ABSTRACT

Bismuth-based Sillen-Aurivillius compounds are being explored as efficient photocatalyst materials for the degradation of organic pollutants due to their unique layered structure that favours effective separation of electron-hole pairs. In this work, we synthesized Sillen-Aurivillius-related Bi2YO4Cl with the bandgap of 2.5 eV by a simple solid-state reaction and sensitized with rhodium nickel (RhNi) nanoparticles (NPs) to form the RhNi/Bi2YO4Cl heterostructure. Photocatalytic activities of BiOCl, Bi2YO4Cl and the RhNi/Bi2YO4Cl heterostructure were examined for the degradation of rhodamine- 6G under visible-light illumination. Results demonstrated that the photocatalytic dye degradation efficiency of RhNi/Bi2YO4Cl heterostructures is higher than those of BiOCl and Bi2YO4Cl, attributed to the synergistic molecular-scale alloying effect of bimetallic RhNi NPs. The plausible mechanism for the degradation of rhodamine-6G and the effective electron-hole pair utilization mechanism were discussed. More... »

PAGES

405-414

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11706-018-0435-y

DOI

http://dx.doi.org/10.1007/s11706-018-0435-y

DIMENSIONS

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