Preparation of polypyrrole/multi-walled carbon nanotube hybrids by electropolymerization combined with a coating method for counter electrodes in dye-sensitized solar cells View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-07

AUTHORS

Jaroslav Kuliček, Pavol Gemeiner, Mária Omastová, Matej Mičušík

ABSTRACT

In this work, multi-wall carbon nanotubes coated with polypyrrole (PPy/MWCNT) have been used as counter electrode (CE) materials for dye-sensitized solar cells (DSSCs). PPy was deposited onto fluorine-doped tin-oxide-coated glass by electrochemical polymerization of pyrrole. Three surfactants were used in the preparation of the hybrids: cationic cetyltrimethylammonium bromide, anionic sodium dodecylbenzenesulfonate (DBSNa), and non-ionic polyoxyethylene sorbitan monolaurate (Tween20). The morphologies of the PPy and PPy/MWCNT hybrids were investigated using scanning electron spectroscopy. Chemical composition of the prepared CEs was determined by X-ray photoelectron spectroscopy and Fourier-transformed infrared spectroscopy. The catalytic activity of the PPy and PPy/MWCNT layers was evaluated using cyclic voltammetry, and the photovoltaic properties of DSSCs with PPy and PPy/MWCNT CEs were characterized using I–V measurements. PPy/MWCNT samples that were prepared by electrochemical polymerization showed the best results when the anionic surfactant DBSNa was used during polymerization. The photoelectric conversion efficiency of PPy/MWCNT prepared by electrochemical polymerization was 2.9%, which was 59% of that of Pt CE (4.9%). More... »

PAGES

1651-1667

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11696-018-0476-9

DOI

http://dx.doi.org/10.1007/s11696-018-0476-9

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