Direct Comparison of Thermoelectric Devices Using Impedance Spectroscopy View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2019-04

AUTHORS

Chung-Yul Yoo, Hana Yoon, Sang Hyun Park

ABSTRACT

The thermoelectric properties of devices based on bismuth telluride, skutterudite, and calcium manganese oxide have been investigated and compared using impedance spectroscopy at 23°C. Prior to the detailed analysis, Kramers–Kronig transformation tests were performed to examine the validity of the obtained impedance spectra. All the spectra were Kramers–Kronig transformable, and were interpreted using equivalent circuit fitting. The three key parameters (Seebeck coefficient, thermal conductivity, and electrical conductivity) and dimensionless figure of merit of bismuth telluride and skutterudite-based devices were successfully extracted from their respective impedance spectra. However, the thermal conductivity of the calcium manganese oxide-based device was overestimated, while the Seebeck coefficient and electrical conductivity values were reasonably accurate owing to their negligible thermoelectric effect at 23°C. We further proposed that the thermoelectric capacitance obtained from the impedance spectra could be a quantitative measure of the “propensity” of thermoelectric devices to generate thermoelectric power under an external temperature gradient. More... »

PAGES

1833-1839

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11664-018-6777-5

DOI

http://dx.doi.org/10.1007/s11664-018-6777-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1109784527


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