High-Temperature Transport Properties of Colusite Cu24T2V2Ge6S32 (T = Ni, Co) View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2017-05

AUTHORS

Y. Bouyrie, V. Ohorodniichuk, S. Sassi, P. Masschelein, A. Dauscher, C. Candolfi, B. Lenoir

ABSTRACT

Sulfur-based minerals have emerged as interesting candidates for thermoelectric applications at high temperatures, with tetrahedrites and colusites being two prominent examples. Here, we extend the investigations on the latter family by reporting on the synthesis and the high-temperature thermoelectric properties of two polycrystalline colusites, Cu24Ni2V2Ge6S32 and Cu24Co2V2Ge6S32. Both samples were prepared by powder metallurgy and consolidated by spark plasma sintering. Successful substitution of Ni and Co for Cu was confirmed by powder x-ray diffraction and scanning electron microscopy which further revealed a homogeneous distribution of the elements within the colusite matrix. The electrical resistivity and thermopower values measured in the Ni sample indicate a more pronounced metallic character with respect to the Co sample. These two samples exhibit very low lattice thermal conductivities of the order of 0.5 W m−1 K−1 at 690 K. Despite this remarkable property, the Ni and Co concentrations studied here did not give rise to enhanced ZT values relative to the previously reported parent compound Cu26V2Ge6S32, with a peak ZT value of 0.5 at 690 K achieved in the Ni sample. More... »

PAGES

2684-2690

References to SciGraph publications

Journal

TITLE

Journal of Electronic Materials

ISSUE

5

VOLUME

46

Author Affiliations

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11664-016-4893-7

DOI

http://dx.doi.org/10.1007/s11664-016-4893-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1030146321


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