High-Temperature Transport Properties of Yb4−xSmxSb3 View Full Text


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Article Info

DATE

2010-09

AUTHORS

A. Chamoire, F. Gascoin, C. Estournès, T. Caillat, J.-C. Tédenac

ABSTRACT

Polycrystalline L4Sb3 (L = La, Ce, Sm, and Yb) and Yb4−xSmxSb3, which crystallizes in the anti-Th3P4 structure type (I-43d no. 220), were synthesized via high-temperature reaction. Structural and chemical characterization were performed by x-ray diffraction and electronic microscopy with energy-dispersive x-ray analysis. Pucks were densified by spark plasma sintering. Transport property measurements showed that these compounds are n-type with low Seebeck coefficients, except for Yb4Sb3, which shows semimetallic behavior with hole conduction above 523 K. By partially substituting Yb by a trivalent rare earth we successfully improved the thermoelectric figure of merit of Yb4Sb3 up to 0.7 at 1273 K. More... »

PAGES

1579-1582

References to SciGraph publications

  • 1977. Intermediate Valence Properties of a Series of Ln4X3 Compounds with Anti-Th3P4 Structure in VALENCE INSTABILITIES AND RELATED NARROW-BAND PHENOMENA
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    http://scigraph.springernature.com/pub.10.1007/s11664-010-1274-5

    DOI

    http://dx.doi.org/10.1007/s11664-010-1274-5

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