Ontology type: schema:ScholarlyArticle
2018-04-17
AUTHORS ABSTRACTPrenucleation refers to the phenomenon of atomic ordering in the liquid adjacent to the substrate/liquid interface at temperatures above the liquidus. In this paper, we have systematically investigated and holistically quantified the prenucleation phenomenon as a function of temperature and the lattice misfit between the substrate and the solid, using molecular dynamics (MD) simulations. Our results have confirmed that at temperatures above the liquidus, the atoms in the liquid at the interface may exhibit pronounced atomic ordering, manifested by atomic layering normal to the interface, in-plane atomic ordering parallel to the interface, and the formation of a 2-dimensional (2D) ordered structure (a few atomic layers in thickness) on the substrate surface. Holistic quantification of such atomic ordering at the interface has revealed that the atomic layering is independent of lattice misfit and is only slightly enhanced by reducing temperature while both in-plane atomic ordering and the formation of the 2D ordered structure are significantly enhanced by reducing the lattice misfit and/or temperature. This substrate-induced atomic ordering in the liquid may have a significant influence on the subsequent heterogeneous nucleation process. More... »
PAGES2766-2777
http://scigraph.springernature.com/pub.10.1007/s11661-018-4628-x
DOIhttp://dx.doi.org/10.1007/s11661-018-4628-x
DIMENSIONShttps://app.dimensions.ai/details/publication/pub.1103400854
JSON-LD is the canonical representation for SciGraph data.
TIP: You can open this SciGraph record using an external JSON-LD service: JSON-LD Playground Google SDTT
[
{
"@context": "https://springernature.github.io/scigraph/jsonld/sgcontext.json",
"about": [
{
"id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/09",
"inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/",
"name": "Engineering",
"type": "DefinedTerm"
},
{
"id": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/0912",
"inDefinedTermSet": "http://purl.org/au-research/vocabulary/anzsrc-for/2008/",
"name": "Materials Engineering",
"type": "DefinedTerm"
}
],
"author": [
{
"affiliation": {
"alternateName": "BCAST, Brunel University London, UB8 3PH, Uxbridge, Middlesex, UK",
"id": "http://www.grid.ac/institutes/grid.7728.a",
"name": [
"BCAST, Brunel University London, UB8 3PH, Uxbridge, Middlesex, UK"
],
"type": "Organization"
},
"familyName": "Men",
"givenName": "H.",
"id": "sg:person.016175621735.55",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.016175621735.55"
],
"type": "Person"
},
{
"affiliation": {
"alternateName": "BCAST, Brunel University London, UB8 3PH, Uxbridge, Middlesex, UK",
"id": "http://www.grid.ac/institutes/grid.7728.a",
"name": [
"BCAST, Brunel University London, UB8 3PH, Uxbridge, Middlesex, UK"
],
"type": "Organization"
},
"familyName": "Fan",
"givenName": "Z.",
"id": "sg:person.014202761657.20",
"sameAs": [
"https://app.dimensions.ai/discover/publication?and_facet_researcher=ur.014202761657.20"
],
"type": "Person"
}
],
"citation": [
{
"id": "sg:pub.10.1557/mrs2004.261",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1067968632",
"https://doi.org/10.1557/mrs2004.261"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/bf02654921",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1021119879",
"https://doi.org/10.1007/bf02654921"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1038/37069",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1017598205",
"https://doi.org/10.1038/37069"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1023/a:1015824230008",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1002687355",
"https://doi.org/10.1023/a:1015824230008"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1007/s11661-012-1495-8",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1050665841",
"https://doi.org/10.1007/s11661-012-1495-8"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1557/mrs2004.264",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1067968635",
"https://doi.org/10.1557/mrs2004.264"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1038/43141",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1006990270",
"https://doi.org/10.1038/43141"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1038/35059035",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1050863922",
"https://doi.org/10.1038/35059035"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1023/a:1015190207719",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1012230283",
"https://doi.org/10.1023/a:1015190207719"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1038/nature08986",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1053210439",
"https://doi.org/10.1038/nature08986"
],
"type": "CreativeWork"
},
{
"id": "sg:pub.10.1038/35048537",
"sameAs": [
"https://app.dimensions.ai/details/publication/pub.1012700890",
"https://doi.org/10.1038/35048537"
],
"type": "CreativeWork"
}
],
"datePublished": "2018-04-17",
"datePublishedReg": "2018-04-17",
"description": "Prenucleation refers to the phenomenon of atomic ordering in the liquid adjacent to the substrate/liquid interface at temperatures above the liquidus. In this paper, we have systematically investigated and holistically quantified the prenucleation phenomenon as a function of temperature and the lattice misfit between the substrate and the solid, using molecular dynamics (MD) simulations. Our results have confirmed that at temperatures above the liquidus, the atoms in the liquid at the interface may exhibit pronounced atomic ordering, manifested by atomic layering normal to the interface, in-plane atomic ordering parallel to the interface, and the formation of a 2-dimensional (2D) ordered structure (a few atomic layers in thickness) on the substrate surface. Holistic quantification of such atomic ordering at the interface has revealed that the atomic layering is independent of lattice misfit and is only slightly enhanced by reducing temperature while both in-plane atomic ordering and the formation of the 2D ordered structure are significantly enhanced by reducing the lattice misfit and/or temperature. This substrate-induced atomic ordering in the liquid may have a significant influence on the subsequent heterogeneous nucleation process.",
"genre": "article",
"id": "sg:pub.10.1007/s11661-018-4628-x",
"inLanguage": "en",
"isAccessibleForFree": false,
"isFundedItemOf": [
{
"id": "sg:grant.2782533",
"type": "MonetaryGrant"
},
{
"id": "sg:grant.4576283",
"type": "MonetaryGrant"
}
],
"isPartOf": [
{
"id": "sg:journal.1136292",
"issn": [
"1073-5623",
"1543-1940"
],
"name": "Metallurgical and Materials Transactions A",
"publisher": "Springer Nature",
"type": "Periodical"
},
{
"issueNumber": "7",
"type": "PublicationIssue"
},
{
"type": "PublicationVolume",
"volumeNumber": "49"
}
],
"keywords": [
"lattice misfit",
"substrate/liquid interface",
"atomic layering",
"plane atomic ordering",
"atomic ordering",
"substrate surface",
"crystalline substrates",
"heterogeneous nucleation process",
"liquid interface",
"function of temperature",
"nucleation process",
"interface",
"temperature",
"liquid",
"holistic quantification",
"dynamics simulations",
"misfit",
"prenucleation",
"significant influence",
"liquidus",
"molecular dynamics simulations",
"substrate",
"layering",
"simulations",
"surface",
"structure",
"phenomenon",
"plane",
"formation",
"ordering",
"influence",
"process",
"results",
"quantification",
"atoms",
"function",
"paper"
],
"name": "Prenucleation Induced by Crystalline Substrates",
"pagination": "2766-2777",
"productId": [
{
"name": "dimensions_id",
"type": "PropertyValue",
"value": [
"pub.1103400854"
]
},
{
"name": "doi",
"type": "PropertyValue",
"value": [
"10.1007/s11661-018-4628-x"
]
}
],
"sameAs": [
"https://doi.org/10.1007/s11661-018-4628-x",
"https://app.dimensions.ai/details/publication/pub.1103400854"
],
"sdDataset": "articles",
"sdDatePublished": "2022-05-20T07:34",
"sdLicense": "https://scigraph.springernature.com/explorer/license/",
"sdPublisher": {
"name": "Springer Nature - SN SciGraph project",
"type": "Organization"
},
"sdSource": "s3://com-springernature-scigraph/baseset/20220519/entities/gbq_results/article/article_760.jsonl",
"type": "ScholarlyArticle",
"url": "https://doi.org/10.1007/s11661-018-4628-x"
}
]Download the RDF metadata as: json-ld nt turtle xml License info
JSON-LD is a popular format for linked data which is fully compatible with JSON.
curl -H 'Accept: application/ld+json' 'https://scigraph.springernature.com/pub.10.1007/s11661-018-4628-x'
N-Triples is a line-based linked data format ideal for batch operations.
curl -H 'Accept: application/n-triples' 'https://scigraph.springernature.com/pub.10.1007/s11661-018-4628-x'
Turtle is a human-readable linked data format.
curl -H 'Accept: text/turtle' 'https://scigraph.springernature.com/pub.10.1007/s11661-018-4628-x'
RDF/XML is a standard XML format for linked data.
curl -H 'Accept: application/rdf+xml' 'https://scigraph.springernature.com/pub.10.1007/s11661-018-4628-x'
This table displays all metadata directly associated to this object as RDF triples.
150 TRIPLES
22 PREDICATES
73 URIs
54 LITERALS
6 BLANK NODES