Physicochemical properties and gasification reactivity of the ultrafine semi-char derived from a bench-scale fluidized bed gasifier View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2017-08

AUTHORS

Yukui Zhang, Haixia Zhang, Zhiping Zhu, Yongjie Na, Qinggang Lu

ABSTRACT

Zhundong coalfield is the largest intact coalfield worldwide and fluidized bed gasification has been considered as a promising way to achieve its clean and efficient utilization. The purpose of this study is to investigate the physicochemical properties and gasification reactivity of the ultrafine semi-char, derived from a bench-scale fluidized bed gasifier, using Zhundong coal as fuel. The results obtained are as follows. In comparison to the raw coal, the carbon and ash content of the semi-char increase after partial gasification, but the ash fusion temperatures of them show no significant difference. Particularly, 76.53% of the sodium in the feed coal has released to the gas phase after fluidized bed gasification. The chemical compositions of the semi-char are closely related to its particle size, attributable to the distinctly different natures of diverse elements. The semi-char exhibits a higher graphitization degree, higher BET surface area, and richer meso- and macropores, which results in superior gasification reactivity than the coal char. The chemical reactivity of the semi-char is significantly improved by an increased gasification temperature, which suggests the necessity of regasification of the semi-char at a higher temperature. Consequently, it will be considered feasible that these carbons in the semi-char from fluidized bed gasifiers are reclaimed and reused for the gasification process. More... »

PAGES

362-370

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11630-017-0950-7

DOI

http://dx.doi.org/10.1007/s11630-017-0950-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1090741860


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