Sulfate radical-mediated degradation of phenol and methylene blue by manganese oxide octahedral molecular sieve (OMS-2) activation of peroxymonosulfate View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2019-03-20

AUTHORS

Jing Wei, Xiaoming Li, Qi Yang, You Wu, Xiaoding Huang, Ziletao Tao, Qiuxiang Xu, Xiaofei Zhu, Dongbo Wang

ABSTRACT

Activation of peroxymonosulfate (PMS) has been concentrated on degrading refractory organic pollutants owing to the generation of sulfate radical (SO4•−\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$ S{O}_4^{\bullet -} $$\end{document}) with high standard redox potential. In this study, manganese oxide octahedral molecular sieve (OMS-2) with cryptomelane type was synthesized by a new hydrothermal method to activate PMS for the degradation of phenol and methylene blue (MB) in water. The as-prepared composites were fully characterized, and the effects of PMS dosage, OMS-2 dosage, initial pollutant concentration, pH, and chloride on the degradation of phenol were elaborately investigated. Moreover, the phenol degradation was evaluated through the variations of total organic carbon (TOC) and three-dimensional excitation emission matrix (3D-EEM), and reaction intermediates were also investigated. Both electron spin resonance (ESR) spectra and comparative experiments suggested SO4•−\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$ S{O}_4^{\bullet -} $$\end{document} and hydroxyl radical (HO•) took part in the phenol degradation and SO4•−\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$ S{O}_4^{\bullet -} $$\end{document} was more significant than HO•. The fine degradation efficiency of phenol in different water source, as well as the stability after continuous use, indicated the possible application of PMS/OMS-2 in real wastewater treatment. More... »

PAGES

12963-12974

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11356-019-04749-3

DOI

http://dx.doi.org/10.1007/s11356-019-04749-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1112895782

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30895542


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