Efficient decomposition of perchlorate to chloride ions in subcritical water by use of steel slag View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2018-03

AUTHORS

Hisao Hori, Ayae Kamijo, Miki Inoue, Asako Chino, Qian Wu, Kurunthachalam Kannan

ABSTRACT

Decomposition of perchlorate (ClO4-) in subcritical water in the presence of steel slag, a by-product of the steel industry, was investigated. Reactivity of ClO4- was low in pure subcritical water state up to 300 °C, whereas adding steel slag efficiently accelerated the decomposition of ClO4- to Cl-, with no leaching of heavy metals such as chromium and other environmentally undesirable elements (boron and fluorine). When the reaction was performed in subcritical water at a relatively low temperature (250 °C) for 6 h, virtually all ClO4- ions were removed from the reaction solution. The concentration of Cl- after the reaction was well accounted for by the sum of the amount of Cl- ascribed to the decomposition of ClO4- and the amount of Cl- leached from the slag. This method was successfully applied to decompose ClO4- in water samples collected from a man-made reflection pond following a fireworks display, even though these samples contained much higher concentrations of Cl- and SO42- than ClO4-. More... »

PAGES

7262-7270

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11356-016-7332-7

DOI

http://dx.doi.org/10.1007/s11356-016-7332-7

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1049616886

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/27488707


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43 schema:description Decomposition of perchlorate (ClO<sub>4</sub><sup>-</sup>) in subcritical water in the presence of steel slag, a by-product of the steel industry, was investigated. Reactivity of ClO<sub>4</sub><sup>-</sup> was low in pure subcritical water state up to 300 °C, whereas adding steel slag efficiently accelerated the decomposition of ClO<sub>4</sub><sup>-</sup> to Cl<sup>-</sup>, with no leaching of heavy metals such as chromium and other environmentally undesirable elements (boron and fluorine). When the reaction was performed in subcritical water at a relatively low temperature (250 °C) for 6 h, virtually all ClO<sub>4</sub><sup>-</sup> ions were removed from the reaction solution. The concentration of Cl<sup>-</sup> after the reaction was well accounted for by the sum of the amount of Cl<sup>-</sup> ascribed to the decomposition of ClO<sub>4</sub><sup>-</sup> and the amount of Cl<sup>-</sup> leached from the slag. This method was successfully applied to decompose ClO<sub>4</sub><sup>-</sup> in water samples collected from a man-made reflection pond following a fireworks display, even though these samples contained much higher concentrations of Cl<sup>-</sup> and SO<sub>4</sub><sup>2-</sup> than ClO<sub>4</sub><sup>-</sup>.
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