Photocatalytic abatement results from a model street canyon View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2015-11

AUTHORS

M. Gallus, R. Ciuraru, F. Mothes, V. Akylas, F. Barmpas, A. Beeldens, F. Bernard, E. Boonen, A. Boréave, M. Cazaunau, N. Charbonnel, H. Chen, V. Daële, Y. Dupart, C. Gaimoz, B. Grosselin, H. Herrmann, S. Ifang, R. Kurtenbach, M. Maille, I. Marjanovic, V. Michoud, A. Mellouki, K. Miet, N. Moussiopoulos, L. Poulain, P. Zapf, C. George, J. F. Doussin, J. Kleffmann

ABSTRACT

During the European Life+ project PhotoPAQ (Demonstration of Photocatalytic remediation Processes on Air Quality), photocatalytic remediation of nitrogen oxides (NOx), ozone (O3), volatile organic compounds (VOCs), and airborne particles on photocatalytic cementitious coating materials was studied in an artificial street canyon setup by comparing with a colocated nonactive reference canyon of the same dimension (5 × 5 × 53 m). Although the photocatalytic material showed reasonably high activity in laboratory studies, no significant reduction of NOx, O3, and VOCs and no impact on particle mass, size distribution, and chemical composition were observed in the field campaign. When comparing nighttime and daytime correlation plots of the two canyons, an average upper limit NOx remediation of ≤2% was derived. This result is consistent only with three recent field studies on photocatalytic NOx remediation in the urban atmosphere, whereas much higher reductions were obtained in most other field investigations. Reasons for the controversial results are discussed, and a more consistent picture of the quantitative remediation is obtained after extrapolation of the results from the various field campaigns to realistic main urban street canyon conditions. More... »

PAGES

18185-18196

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11356-015-4926-4

DOI

http://dx.doi.org/10.1007/s11356-015-4926-4

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1027425545

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26178827


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424 rdf:type schema:Organization
425 https://www.grid.ac/institutes/grid.462054.1 schema:alternateName Institute of Researches on Catalysis and Environment in Lyon
426 schema:name Université de Lyon, Université Lyon 1, CNRS, UMR5256, IRCELYON, Institut de recherches sur la catalyse et l’environnement de Lyon, F-69626, Villeurbanne, France
427 rdf:type schema:Organization
428 https://www.grid.ac/institutes/grid.462466.4 schema:alternateName Institut de Combustion Aérothermique Réactivité et Environnement
429 schema:name Institut de Combustion, Aérothermique, Réactivité et Environnement (ICARE), CNRS (UPR 3021)/OSUC, 1C Avenue de la Recherche Scientifique, Orléans, France
430 rdf:type schema:Organization
431 https://www.grid.ac/institutes/grid.464159.b schema:alternateName Laboratoire Interuniversitaire des Systèmes Atmosphériques
432 schema:name LISA, UMR CNRS 7583, Université Paris Est Créteil et Université Paris Diderot, Institut Pierre Simon Laplace, Créteil, France
433 rdf:type schema:Organization
434 https://www.grid.ac/institutes/grid.4793.9 schema:alternateName Aristotle University of Thessaloniki
435 schema:name Laboratory of Heat Transfer and Environmental Engineering (LHTEE), Aristotle University of Thessaloniki, Box 483, GR 54124, Thessaloniki, Greece
436 rdf:type schema:Organization
437 https://www.grid.ac/institutes/grid.7787.f schema:alternateName University of Wuppertal
438 schema:name Physikalische und Theoretische Chemie/FB C, Bergische Universität Wuppertal (BUW), Gaußstr. 20, 42119, Wuppertal, Germany
439 rdf:type schema:Organization
 




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