Investigation of uranium binding forms in selected German mineral waters View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2013-12

AUTHORS

Alfatih A. A. Osman, Gerhard Geipel, Gert Bernhard, Eckhard Worch

ABSTRACT

Cryogenic time-resolved laser-induced fluorescence spectroscopy was successfully used to identify uranium binding forms in selected German mineral waters of extremely low uranium concentrations (<2.0 μg/L). The measurements were performed at a low temperature of 153 K. The spectroscopic data showed a prevalence of aquatic species Ca2UO2(CO3)3 in all investigated waters, while other uranyl-carbonate complexes, viz, UO2CO3(aq) and UO2(CO3)2 (2-), only existed as minor species. The pH value, alkalinity (CO3 (2-)), and the main water inorganic constituents, specifically the Ca(2+) concentration, showed a clear influence on uranium speciation. Speciation modeling was performed using the most recent thermodynamic data for aqueous complexes of uranium. The modeling results for the main uranium binding form in the investigated waters indicated a good agreement with the spectroscopy measurements. More... »

PAGES

8629-8635

References to SciGraph publications

  • 2006. LASER-INDUCED FLUORESCENCE SPECTROSCOPY in HANDBOOK OF APPLIED SOLID STATE SPECTROSCOPY
  • 2011. Uranium in German Tap and Groundwater – Occurrence and Origins in THE NEW URANIUM MINING BOOM
  • Identifiers

    URI

    http://scigraph.springernature.com/pub.10.1007/s11356-013-1822-7

    DOI

    http://dx.doi.org/10.1007/s11356-013-1822-7

    DIMENSIONS

    https://app.dimensions.ai/details/publication/pub.1032841987

    PUBMED

    https://www.ncbi.nlm.nih.gov/pubmed/23702572


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