Neutron Insights into Sorption Enhanced Methanol Catalysis View Full Text


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Article Info

DATE

2021-06-06

AUTHORS

Marin Nikolic, Luke Daemen, Anibal J. Ramirez-Cuesta, Rafael Balderas Xicohtencatl, Yongqiang Cheng, Seth T. Putnam, Nicholas P. Stadie, Xiaochun Liu, Jasmin Terreni, Andreas Borgschulte

ABSTRACT

Sorption enhanced methanol production makes use of the equilibrium shift of the CO2\documentclass[12pt]{minimal} \usepackage{amsmath} \usepackage{wasysym} \usepackage{amsfonts} \usepackage{amssymb} \usepackage{amsbsy} \usepackage{mathrsfs} \usepackage{upgreek} \setlength{\oddsidemargin}{-69pt} \begin{document}$$\hbox {CO}_2$$\end{document} hydrogenation reaction towards the desired products. However, the increased complexity of the catalyst system leads to additional reactions and thus side products such as dimethyl ether, and complicates the analysis of the reaction mechanism. On the other hand, the unusually high concentration of intermediates and products in the sorbent facilitates the use of inelastic neutron scattering (INS) spectroscopy. Despite being a post-mortem method, the INS data revealed the change of the reaction path during sorption catalysis. Concretely, the experiments indicate that the varying water partial pressure due to the adsorption saturation of the zeolite sorbent influences the progress of the reaction steps in which water is involved. Experiments with model catalysts support the INS findings. More... »

PAGES

638-643

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11244-021-01461-w

DOI

http://dx.doi.org/10.1007/s11244-021-01461-w

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1138645828

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/34720545


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