NSR Catalysis studied using Scanning Tunnelling Microscopy View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2007-05

AUTHORS

Michael Bowker, Marco Cristofolini, Matt Hall, Elodie Fourre, Federico Grillo, Elin McCormack, Peter Stone, Masaru Ishii

ABSTRACT

In this paper we report the fabrication of model catalysts prepared to understand the structure of the BaO surface. This utilises the ‘inverse’ catalyst method, that is, the oxide layer is fabricated onto the top of a metal single crystal surface. We show that we can atomically resolve the surface structure of BaO(111) and that it presents a (2×2) reconstruction at its surface. Under other dosing conditions we can produce a layer which is metastable at 573K, which we believe to be the peroxide, BaO2. We have shown that the BaO layer can store NOx from a mix of NO and oxygen, even under the extremely low exposure conditions of UHV, proving that the NOx storage process is a facile one. The results indicate that it is not necessary to have NO2 in the gas phase in order to store NOx. More... »

PAGES

341-343

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11244-007-0202-2

DOI

http://dx.doi.org/10.1007/s11244-007-0202-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1049699448


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140 https://www.grid.ac/institutes/grid.5600.3 schema:alternateName Cardiff University
141 schema:name Wolfson Nanoscience Laboratory, School of Chemistry, Cardiff University, CF10 3AT, Cardiff, UK
142 rdf:type schema:Organization
 




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