Stereo sensitivity of exchange interactions in NiII and CuII heterospin complexes with 5-formylpyrrolyl-substituted nitroxides View Full Text


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Article Info

DATE

2016-03

AUTHORS

E. M. Zueva, E. V. Tretyakov, S. V. Fokin, G. V. Romanenko, A. O. Tkacheva, A. S. Bogomyakov, O. V. Petrova, B. A. Trofimov, R. Z. Sagdeev, V. I. Ovcharenko

ABSTRACT

5-Formylpyrrolyl-substituted nitronyl and imino nitroxide radicals HL1 and HL2 were synthesized. Their solid phases are formed by packing pairs of the molecules. In the {HL1...HL1} pairs, the dominant interaction is the ferromagnetic exchange with J/kB = 8.8 K (Hamiltonian H=2J(s1→·s2→)). The ferromagnetic exchange occurs also in the heterospin molecules [Ni(L1)2], [Cu(L1)2], and [Ni(L2)2(MeOH)2]. In the complexes [Ni(L1)2] and [Cu(L1)2], a small change in the mutual orientation of the coordinated ligands has a considerable effect on the value and the sign of the energy of exchange interactions between the unpaired electrons of the metal ion and paramagnetic ligands. More... »

PAGES

666-674

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11172-016-1353-8

DOI

http://dx.doi.org/10.1007/s11172-016-1353-8

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https://app.dimensions.ai/details/publication/pub.1013844715


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