Binuclear copper(ii) and nickel(ii) complexes based on N,N′-bis(3-formyl-5-tert-butylsalicylidene)-1,3-diaminopropan-2-ol: physicochemical and theoretical study View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2014-03

AUTHORS

S. I. Levchenkov, I. N. Shcherbakov, L. D. Popov, Yu. P. Tupolova, K. Yu. Suponitskii, M. I. Mazuritskii, V. A. Kogan

ABSTRACT

Binuclear CuII and NiII complexes with exogenous acetate and pyrazolate bridges were synthesized and studied. It was shown that the μ2-coordination of the DMSO molecule in an acetate-bridged CuII complex leads to the inversion of the sign of the exchange interaction parameter. Quantum chemical calculations of the geometry of the complexes and the magnetic exchange parameters showed that the role of the DMSO molecule is to stabilize the “distorted” conformation of metallocycles. More... »

PAGES

673-683

References to SciGraph publications

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  • 2010-02. Molecular design of azomethine complexes in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • 2011-07-03. Crystal structure and magnetic properties of the binuclear copper(II) complex based on 1,3-diaminopropan-2-ol N,N′-bis(3-formyl-5-tert-butylsalicylidene) in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • 2008-10-14. New ferro-and antiferromagnetic complexes of tridentate azomethines with copper in RUSSIAN JOURNAL OF INORGANIC CHEMISTRY
  • 2010-03. Quantum chemical interpretation of different types of exchange magnetic interactions in dinuclear copper azomethine chelates in RUSSIAN CHEMICAL BULLETIN
  • 2010-11. Physicochemical study of new polydentane ligand systems based on 2,6-diformyl-4-tert-butylphenol in RUSSIAN JOURNAL OF GENERAL CHEMISTRY
  • 2009-12. 1-Hydrazinophthalazine based hydrazones and their transition metal complexes: Structure and biological activity in RUSSIAN JOURNAL OF GENERAL CHEMISTRY
  • 2005-03. Dinuclear copper(II) complexes with an unsymmetrical exchange fragment in RUSSIAN CHEMICAL BULLETIN
  • 2009-08-21. Influence of structural factors on the magnetic properties of the binuclear copper complexes with salicylaldehyde hydrazone and bis(hydrazone)-2,6-diformylphenol: Quantum-chemical calculations in RUSSIAN JOURNAL OF COORDINATION CHEMISTRY
  • 2008-09-25. Theoretical study on the magnetic exchange behavior of a hetero-double-bridged binuclear copper(II) complex: orbital complementary effect in TRANSITION METAL CHEMISTRY
  • 2001-04. Quantum computing in molecular magnets in NATURE
  • 2007-06-07. Synthesis and magnetic properties of the novel binuclear copper(II) metallochelates with unsymmetrical exchange fragment including heterocyclic derivatives in TRANSITION METAL CHEMISTRY
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