Modern concepts on catalysis of hydroprocessing and synthesis of alcohols from syngas by transition metal sulfides View Full Text


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Article Info

DATE

2014-02

AUTHORS

V. M. Kogan, P. A. Nikul’shin, V. S. Dorokhov, E. A. Permyakov, A. V. Mozhaev, D. I. Ishutenko, O. L. Eliseev, N. N. Rozhdestvenskaya, A. L. Lapidusa

ABSTRACT

A concept on the dynamic nature of active centers (AC) of the catalysts based on transition metal sulfides is described. The concept formed the basis of a “dynamic” model, according to which AC formed and functioning under the reaction conditions can oscillate between layers of promoted molybdenum sulfide. The model assumes the existence of “rapid” and “slow” AC and the possibility of their intertransformation due to the reversible migration of sulfur and promoter between the crystallite layers in a hydrogen atmosphere. The frequency of these migrations (oscillations) determines the catalyst activity. An assumption is substantiated that the hydrogenation sites are localized at the rims of Co(Ni)MoS2 crystallites and desulfurization (hydrodesulfurization) sites are localized on the edges. The proposed model makes it possible to develop criteria for the evaluation of the efficiency of catalytic performance for hydrodesulfurization of hydrocarbon raw materials of various types and for synthesis of higher alcohols from syngas. More... »

PAGES

332-345

References to SciGraph publications

  • 2013-07. The mechanism of synthesis gas conversion to alcohols catalyzed by transition metal sulfides in DOKLADY CHEMISTRY
  • 2005-01. 35S Tracer study of the effect of support nature on the dynamics of the active sites of CoMo and NiMo sulfide catalysts supported on Al 2O3 and activated carbon in KINETICS AND CATALYSIS
  • 2011-11-30. Cobalt salts of decamolybdodicobaltic acid as precursors of the highly reactive type II CoMoS phase in hydrorefining catalysts in KINETICS AND CATALYSIS
  • 2012-09-27. Influence of the composition and morphology of nanosized transition metal sulfides prepared using the Anderson-type heteropoly compounds [X(OH)6Mo6O18]n− (X = Co, Ni, Mn, Zn) and [Co2Mo10O38H4]6− on their catalytic properties in KINETICS AND CATALYSIS
  • 1990-03. Investigation of the promotion effect on the sulfide sulfur mobility and on the catalytic activity of hydrotreating Co/Mo/Al2O3 catalysts using35S in CATALYSIS LETTERS
  • 2008-03. Influence of Anderson and Keggin heteropoly compounds as precursors of oxide phases in hydrotreating catalysts on their performance in PETROLEUM CHEMISTRY
  • 2003-07. In Situ Radioisotopic Study of the Active Sites of Sulfide CoMo Catalysts and the Mechanism of Thiophene Hydrodesulfurization in KINETICS AND CATALYSIS
  • 1996. Hydrotreating Catalysis in CATALYSIS
  • 2012-01-26. Activity of Co(Ni)MoS/Al2O3 catalysts, derived from cobalt(nickel) salts of H6[Co2Mo10O38H4], in hydrogenolysis of thiophene and hydrogen treatment of diesel fraction in PETROLEUM CHEMISTRY
  • 2013-03. Conversion of synthesis gas into alcohols on supported cobalt-molybdenum sulfide catalysts promoted with potassium in KINETICS AND CATALYSIS
  • 2009-03. Thiophene hydrodesulfurization and diesel fuel hydrorefining activities of XMo6(S)/γ-Al2O3 and Ni-XMo6(S)/γ-Al2O3 (X = Al, Ga, In, Fe, Co, and Ni) catalysts in KINETICS AND CATALYSIS
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    http://scigraph.springernature.com/pub.10.1007/s11172-014-0434-9

    DOI

    http://dx.doi.org/10.1007/s11172-014-0434-9

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    https://app.dimensions.ai/details/publication/pub.1029177978


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