Conversion of ethanol into hydrocarbon components of fuels in the presence of Pd-Zn-containing catalysts View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2014-01

AUTHORS

A. V. Chistyakov, M. A. Gubanov, V. Yu. Murzin, P. A. Zharova, M. V. Tsodikov, V. V. Kriventsov, A. E. Gekhman, I. I. Moiseev

ABSTRACT

The features of ethanol conversion into hydrocarbons C4-C12 in the presence of the novel catalyst Pd-Zn/γ-alumina and pilot zeolite system Pd-Zn/MFI/γ-alumina were studied (MFI is high-siliceous zeolite with ZSM-5 type structure). The structure of active sites changes noticeably in the course of preliminary activation and catalytic reaction. High selectivity and stability of the zeolite-containing Pd-Zn catalyst in alcohol conversion into hydrocarbon components of fuels is related to the stable composition of the alloy that forms clusters PdZn. At the same time, the alumina-based catalyst loses stability due to zinc diffusion from the alloy into γ-Al2O3 to form the spinel structure. More... »

PAGES

88-93

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11172-014-0399-8

DOI

http://dx.doi.org/10.1007/s11172-014-0399-8

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1020590166


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