Effect of Pt nanoparticle size on the specific catalytic activity of Pt/SiO2 and Pt/TiO2 in the total oxidation of methane ... View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2010-09

AUTHORS

A. Yu. Stakheev, A. M. Gololobov, I. E. Beck, G. O. Bragina, V. I. Zaikovsky, A. B. Ayupov, N. S. Telegina, V. I. Bukhtiyarov

ABSTRACT

The dependence of the specific catalytic activity (Asp) of the catalysts Pt/SiO2 and Pt/TiO2 in the total oxidation of CH4 and n-C4H10 on the Pt nanoparticle size (in the range from 1 to 4 nm) was studied. The specific catalytic activity increases with an increase in the platinum nanoparticle size, indicating that the total oxidation is a structure-sensitive reaction. The structure sensitivity depends on the size of an oxidized molecule: it increases sharply on going from CH4 to n-C4H10. The support also exerts a considerable effect on the Asp value: in the oxidation of both CH4 and C4H10 the specific catalytic activity for the catalysts Pt/TiO2 is 3–4 times that for Pt/SiO2. More... »

PAGES

1713-1719

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11172-010-0301-2

DOI

http://dx.doi.org/10.1007/s11172-010-0301-2

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1038010274


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