Stability issues of CO tolerant Pt-based electrocatalysts for polymer electrolyte membrane fuel cells: comparison of Pt/Ti0.8Mo0.2O2–C with PtRu/C View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2019-04

AUTHORS

Ádám Vass, Irina Borbáth, István Bakos, Zoltán Pászti, György Sáfrán, András Tompos

ABSTRACT

The stability and CO tolerance of a self-made 20 wt% Pt/Ti0.8Mo0.2O2–C mixed oxide–carbon composite supported electrocatalyst was compared to those of a commercial state-of-the-art PtRu/C electrocatalyst by means of cyclic voltammetry and COads stripping voltammetry measurements. On the Pt/Ti0.8Mo0.2O2–C catalyst the oxidation of CO takes place at exceptionally low potential values (ECO,onset = 50 mV); the onset potential is shifted to less positive potentials by 150 mV compared to the PtRu/C catalyst. A stability test involving 500 polarization cycles revealed that the PtRu/C catalyst suffered more significant degradation than the composite supported Pt catalyst. XPS measurements indicated that the degradation is connected to ruthenium dissolution. At the same time, better electrocatalytic stability and increased CO tolerance of the Pt/Ti0.8Mo0.2O2–C electrocatalyst compared to the PtRu/C catalyst was evidenced. More... »

PAGES

1-21

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11144-018-1512-z

DOI

http://dx.doi.org/10.1007/s11144-018-1512-z

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1110481210


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