Improved photocatalytic activity of Z-scheme β-Bi2O3/Bi2WO6 nanocomposites from band bending of p-n heterojunction View Full Text


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Article Info

DATE

2020-05-15

AUTHORS

C. X. Li, S. Y. Song, D. S. Shi, Y. Ying, X. X. Zhang, J. Q. Wei, B. Hong, J. C. Xu, H. X. Jin, P. F. Wang, X. Q. Wang

ABSTRACT

Photocatalytic β-Bi2O3/Bi2WO6 p-n heterojunctions were synthesized by two-step solvothermal method, and then, the phase structure, microstructures, and band structures were characterized with XRD, EDS, N2 adsorption-desorption isotherms, and UV-vis spectroscopy. The β-Bi2O3 nanoparticles with the smaller diameter anchor on the surface of Bi2WO6 nanoparticles to form β-Bi2O3/Bi2WO6 nanocomposites, resulting in the band bending for the balance of Fermi level. The band bending of p-n heterojunctions leads to the Z-scheme β-Bi2O3/Bi2WO6 photocatalysts and electron narrow energy transition between Ec of Bi2WO6 and Ev of β-Bi2O3. The accumulation of electrons at EC of β-Bi2O3 and holes at EV of Bi2WO6 both improve the photocatalytic activity of β-Bi2O3/Bi2WO6 nanocomposites. The photocatalytic removal of ciprofloxacin increases up to about 93% for S-20 with the increasing β-Bi2O3 content under visible light irradiation. Therefore, the β-Bi2O3/Bi2WO6 photocatalysts with the dominant radical of •O2− and holes could be regarded as one of promising candidates in the fields of dealing with antibiotics.Graphical abstract More... »

PAGES

123

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DOI

http://dx.doi.org/10.1007/s11051-020-04873-z

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