Amine-functionalized graphene oxide nanosheets (AFGONs): an efficient bifunctional catalyst for selective formation of 1,4-dihydropyridines, acridinediones and polyhydroquinolines. View Full Text


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Article Info

DATE

2019-04-06

AUTHORS

Prasun Choudhury, Pranab Ghosh, Basudeb Basu

ABSTRACT

We report here selective formation of functionalized 1,4-dihydropyridines (DHP), acridinediones and polyhydroquinolines in high yields using amine-functionalized graphene oxide nanosheets (AFGONs) as the bifunctional catalyst. The method overcomes the limitations of previous protocols affording a mixture of DHP and pyridine derivatives using graphene oxide as the catalyst. The mild reaction conditions are found compatible with a wide range of functional groups. It is presumed that a cooperative effect between the acidic and basic functionalities present in AFGONs may have exerted high catalytic efficiency as well as prevented further oxidation to pyridine derivatives. A plausible mechanism is proposed on the basis of some control experiments. The reactions can be scaled up conveniently, and the catalyst can be recycled for five consecutive runs without loss of its activity. More... »

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s11030-019-09949-0

DOI

http://dx.doi.org/10.1007/s11030-019-09949-0

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1113283536

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/30955149


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