Investigation of molecular interactions in binary mixture of dimethyl carbonate + N-methylformamide at T = (303.15, 308.15, 313.15 and 318.15) ... View Full Text


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Article Info

DATE

2019-03

AUTHORS

Sk. Beebi, Sk. Md. Nayeem, C. Rambabu

ABSTRACT

Density (ρ) and speed of sound (u) of binary liquid mixtures of dimethyl carbonate and N-methylformamide have been determined at T = (303.15, 308.15, 313.15 and 318.15) K over the entire composition range. Experimental data are used to evaluate excess values of molar volume (VmE), isentropic compressibility (ksE), isothermal compressibility (kTE), intermolecular free length (LfE), acoustic impedance (ZE) and ultrasonic speed (uE). The VE data in the present investigation were analysed by using Prigogine–Flory–Patterson (PFP) theory. Partial and excess partial molar volumes (V¯m,1, V¯m,2), (V¯m,1E, V¯m,2E) and partial and excess partial molar volume of the components at infinite dilution (V¯m,1∞, V¯m,2∞), (V¯m,1E,∞, V¯m,2E,∞) at T = (303.15, 308.15, 313.15, 318.15) K have been calculated. The excess/deviation properties were fitted to Redlich–Kister equation to obtain their coefficients and standard deviations. The present investigation also comprises the acoustic nonlinearity parameter (B/A) in the mixtures and calculation of cohesive energy ΔA, Van der Wall’s constants (a, b) and distance of closest approach (d). Moreover, various semi-empirical relations of ultrasonic speed have been used to correlate the theoretical velocities. FT-IR spectra of pure components and their binaries have been measured at T = 298.15 K. More... »

PAGES

3387-3399

References to SciGraph publications

  • 1989-01. Application of the Prigogine-Flory-Patterson theory part III. Mixtures of a bicyclic compound, benzene, cyclohexane,n-hexane with a cycloalkane, cyclohexene, a cycloalkadiene and benzene in JOURNAL OF SOLUTION CHEMISTRY
  • 2007-10. Density and Refractive Index for Binary Systems of the Ionic Liquid [Bmim][BF4] with Methanol, 1,3-Dichloropropane, and Dimethyl Carbonate in JOURNAL OF SOLUTION CHEMISTRY
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  • 2018-04. Thermo-physicochemical investigation of molecular interactions in binary combination (dimethyl carbonate + methyl benzoate) in JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
  • 2009-04. Volumetric, Viscometric, Ultrasonic, and Refractive Index Properties of Liquid Mixtures of Benzene with Industrially Important Monomers at Different Temperatures in INTERNATIONAL JOURNAL OF THERMOPHYSICS
  • 2014-02. Thermodynamic properties of binary mixtures containing 1-alkanols in JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
  • 2014-02. Molecular interactions between amine and cyclic ketones at different temperatures in JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
  • 2014-10. Densities, viscosities, and excess properties for binary mixtures of ethylene glycol with amides at 308.15 K in JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY
  • 2011-02. Densities and Excess Molar Volumes of Binary and Ternary Mixtures Containing Acetonitrile + Acetophenone + 1,2-Pentanediol: Experimental Data, Correlation and Prediction by PFP Theory and ERAS Model in JOURNAL OF SOLUTION CHEMISTRY
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    DOI

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