The reactivity of cokes in Boudouard–Bell reactions in the context of an Ergun model View Full Text


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Article Info

DATE

2015-11

AUTHORS

Andrzej Mianowski, Tomasz Radko, Tomasz Siudyga

ABSTRACT

In previous studies, a kinetic equation based on the Ergun mechanism and concept presented in 1956 was applied to Boudouard–Bell reactions for granular coke (1–3 mm) in the temperature range T = 1173–1423 K. In contrast to several other works on this subject, the proposed equation was based on only three kinetic constants: k1, the rate constant for the Boudouard reaction; k−1, the rate constant for the Bell reaction; and k3, which is related to the oxy-carbon decomposition and CO desorption process. The dependence of these constants on temperature allows certain values characteristic of the aforementioned processes to be calculated, including activation energy of gasification reaction, enthalpy of disproportionation reaction of gasification and activation energy of desorption process. When k−1 > 0, i.e., the Bell reaction and inhibitory effects occur, the kinetic constant k3 can be determined using a portion of the experimental [CO] versus time data normalized to the maximum contribution of CO in the outlet gases. More... »

PAGES

1013-1021

References to SciGraph publications

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URI

http://scigraph.springernature.com/pub.10.1007/s10973-015-4761-3

DOI

http://dx.doi.org/10.1007/s10973-015-4761-3

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1002498672


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