Fast concentration of dissolved forms of cesium radioisotopes from large seawater samples View Full Text


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Article Info

DATE

2012-08-21

AUTHORS

Jan Kameník, Henrieta Dulaiova, Ferdinand Šebesta, Kamila Šťastná

ABSTRACT

The method developed for cesium concentration from large freshwater samples was tested and adapted for analysis of cesium radionuclides in seawater. Concentration of dissolved forms of cesium in large seawater samples (about 100 L) was performed using composite absorbers AMP-PAN and KNiFC-PAN with ammonium molybdophosphate and potassium–nickel hexacyanoferrate(II) as active components, respectively, and polyacrylonitrile as a binding polymer. A specially designed chromatography column with bed volume (BV) 25 mL allowed fast flow rates of seawater (up to 1,200 BV h−1). The recovery yields were determined by ICP-MS analysis of stable cesium added to seawater sample. Both absorbers proved usability for cesium concentration from large seawater samples. KNiFC-PAN material was slightly more effective in cesium concentration from acidified seawater (recovery yield around 93 % for 700 BV h−1). This material showed similar efficiency in cesium concentration also from natural seawater. The activity concentrations of 137Cs determined in seawater from the central Pacific Ocean were 1.5 ± 0.1 and 1.4 ± 0.1 Bq m−3 for an offshore (January 2012) and a coastal (February 2012) locality, respectively, 134Cs activities were below detection limit (<0.2 Bq m−3). More... »

PAGES

841-846

References to SciGraph publications

  • 2011-05-19. Radioactivity of plutonium isotopes, 137Cs and their ratio in sediment, seawater and biota from the east coast of Peninsular Malaysia in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 2010-08-01. Radioactivity in the Exclusive Economic Zone of east coast Peninsular Malaysia: distribution trends of 137Cs in surface seawater in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 2003-01. Comparison of some commercial and laboratory prepared caesium ion-exchangers in CZECHOSLOVAK JOURNAL OF PHYSICS
  • 1997-04. Distribution of3H,137Cs and239,240Pu in the surface seawater around Korea in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 1990-01. Determination of fission-products and actinides in the Black Sea following the Cherynobyl accident in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 1990-05. Composite ion exchanger with ammonium molybdophosphate and its properties in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 2011-11-15. Constrains in gamma spectrometry analysis of fallout 137Cs in coastal marine environment of Arabian sea in India in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 1997-06. Composite sorbents of inorganic ion-exchangers and polyacrylonitrile binding matrix in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
  • 1999. Application of New Inorganic-Organic Composite Absorbers with Polyacrylonitrile Binding Matrix for Separation of Radionuclides from Liquid Radioactive Wastes in CHEMICAL SEPARATION TECHNOLOGIES AND RELATED METHODS OF NUCLEAR WASTE MANAGEMENT
  • 2001-05. Recent developments in HYPERMET PC in JOURNAL OF RADIOANALYTICAL AND NUCLEAR CHEMISTRY
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    URI

    http://scigraph.springernature.com/pub.10.1007/s10967-012-2007-4

    DOI

    http://dx.doi.org/10.1007/s10967-012-2007-4

    DIMENSIONS

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