Complexation of uranium(VI) with aromatic acids such as hydroxamic and benzoic acid investigated by TRLFS View Full Text


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Article Info

DATE

2008-08

AUTHORS

M. Glorius, H. Moll, G. Geipel, G. Bernhard

ABSTRACT

The complex formation of uranium(VI) with salicylhydroxamic, benzohydroxamic, and benzoic acid was investigated by time-resolved laser-induced fluorescence spectroscopy (TRLFS). We observed in all three systems a decrease in the fluorescence intensity with increasing ligand concentration. All identified complexed uranyl species are of the type MpLqHr. In the uranium(VI)-salicylhydroxamate system a 1: 1 complex with a stability constant of log β111 = 17.34±0.06 and a 1: 2 complex with a stability constant of log β122 = 35.0±0.11 was identified. Also in the uranium(VI)-benzohydroxamate system the stability constants are determined to be log β110 = 7.92±0.11 and log β120 = 16.88±0.49. In the uranium(VI)-benzoate system only a 1: 1 complex is existent with a stability constant of log β110 = 3.56±0.05. More... »

PAGES

371-377

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10967-007-7082-6

DOI

http://dx.doi.org/10.1007/s10967-007-7082-6

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