Mg Deficiency Impacts on Magnetocaloric Behavior of La0.77Mg0.23-x□xMnO3 (0 ≤ × ≤ 0.2) Manganites View Full Text


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Article Info

DATE

2022-09-12

AUTHORS

R. Selmi, W. Cherif, N. M. Ferreira

ABSTRACT

This study aims to investigate the magnetocaloric properties of a La0.77Mg0.23-x□xMnO3 (0 ≤ × ≤ 0.2) series elaborated using a solid-state method and published in Alloys Compd., 738, 2018, 528–539. In our crystallographic study, our compounds display an orthorhombic structure with Pnma group space. The Raman analysis confirms the structure formation of the compounds. The magnetic measurements show that all samples displayed a second-order magnetic phase transition from ferromagnetic to paramagnetic state, which is also supported by Landau's theory. The magnetic entropy change (ΔSM) and the relative cooling power (RCP) of La0.77-x□xMg0.23MnO3 (0 ≤ × ≤ 0.2) samples are determined from their measured magnetization data as a function of the magnetic applied field. At μ0H = 5 T, the maximum value of the magnetic entropy change ΔSmax was found to decrease from 2.59 J/kg.K for x = 0.0 to 0.38 J/kg.K for x = 0.2. Our results indicate that the optimum magnetocaloric effect at H = 5 T occurs for the composition x = 0.0, which makes it a promising material in magnetic refrigeration. More... »

PAGES

3585-3601

References to SciGraph publications

  • 2019-06-03. Effects of non-magnetic Ti4+ ion doping on the structural, magnetic and magnetocaloric properties of La0.65Dy0.05Sr0.3Mn1−xTixO3 compounds in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2022-01-16. Enhanced relative cooling power of lanthanum-deficiency manganites La0.77−xMg0.23MnO3 (0 ≤ x ≤ 0.2): structural, magnetic and magnetocaloric properties in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2018-01-17. Griffiths phase-like and its evolution with calcium-deficiency in La0.65Ca0.35MnO3 system in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2017-06-12. Role of the stability of charge ordering in exchange bias effect in doped manganites in SCIENTIFIC REPORTS
  • 2020-02-27. Electrical and thermal properties of Pr0.6Sr0.4−xAgxMnO3 (x = 0.05 and 0.1) manganite in JOURNAL OF MATERIALS SCIENCE
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  • 2020-11-15. Oxygen deficiency effect on the magnetocaloric and critical phenomena for La0.8□0.2MnO3-Δ (Δ = 0, 0.1 and 0.2) compounds: significant enhancement of relative cooling power in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2021-06-25. Impact of potassium substitution on structural, magnetic, magnetocaloric and magneto-transport properties of Nd0.6Sr0.4−xKxMnO3 (0.0 ≤x≤ 0.2) manganite in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2020-01-01. Large magnetocaloric effect in La0.75Ca0.25–xNaxMnO3 (0 ≤ x ≤ 0.10) manganites in APPLIED PHYSICS A
  • 2020-09-18. Synthesis and investigation of oxygen deficiency effect on electric properties of La0.75Ba0.10Sr0.15FeO2.875-δ (δ = 0.00, 0.125 and 0.25) ferrites in JOURNAL OF MATERIALS SCIENCE: MATERIALS IN ELECTRONICS
  • 2021-08-18. Finite-size effects on the evolution of magnetic correlations and magnetocaloric properties of Pr0.4Bi0.2Sr0.4MnO3 in APPLIED PHYSICS A
  • 2013-10. Structural and mechanical properties of Sr+2-doped bismuth manganite thick films in INTERNATIONAL JOURNAL OF SELF-PROPAGATING HIGH-TEMPERATURE SYNTHESIS
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