Magnetization of Crystalline and Amorphous Phases of R2Ti2O7 and R2Zr2O7 (R = Gd, Dy, Tb) View Full Text


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Article Info

DATE

2020-01-13

AUTHORS

A. V. Kuznetsov, O. A. Churkin, V. V. Popov, I. V. Shchetinin, A. A. Ivanov, A. A. Yastrebtsev, B. R. Gaynanov, A. A. Yaroslavtsev, O. V. Chernysheva, F. d’Acapito, A. Puri, P. A. Alekseev, A. P. Menushenkov

ABSTRACT

We present the study of frustrated magnets R2M2O7, where R = Gd, Dy, Tb and M = Ti, Zr. Magnetic susceptibility χ and low-temperature magnetization of perfectly ordered pyrochlores R2Ti2O7, partially disordered fluorites R2Zr2O7, and their completely disordered amorphous phases were measured and analyzed. We have found that structural disorder weakens the exchange interaction of the rare-earth ions. Magnetic moments of dysprosium and terbium, obtained from nearly saturated magnetization, are slightly affected by the disorder while the gadolinium moment is completely independent of it. The local structure of the compounds, including oxygen environment of the rare-earth ions, is discussed in terms of the influence of the crystal electric field on the magnetic properties of R2M2O7. More... »

PAGES

2395-2404

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10948-019-05388-y

DOI

http://dx.doi.org/10.1007/s10948-019-05388-y

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1124051343


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