Local Noncentrosymmetric Structure of Bi2Sr2CaCu2O8+y by X-ray Magnetic Circular Dichroism at Cu K-Edge XANES View Full Text


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Article Info

DATE

2017-11-15

AUTHORS

Andrey A. Ivanov, Valentin G. Ivanov, Alexey P. Menushenkov, Fabrice Wilhelm, Andrei Rogalev, Alessandro Puri, Boby Joseph, Wei Xu, Augusto Marcelli, Antonio Bianconi

ABSTRACT

The two-dimensional Bi2Sr2CaCu2O8+y (Bi2212), the most studied prototype cuprate superconductor, is a lamellar system made of a stack of two-dimensional corrugated CuO2 bilayers separated by Bi2O2 + ySr2 O2 layers. While the large majority of theories, proposed to interpret unconventional high Tc superconductivity in Bi2Sr2CaCu2O8+y, assume a centrosymmetric tetragonal CuO2 lattice for the [CuO2]Ca[CuO2] bilayer, here, we report new compelling results providing evidence for local noncentrosymmetric symmetry at the Cu atom. We have measured polarized Cu K-edge XANES (X-ray absorption near-edge structure) and the K-edge X-ray magnetic circular dichroism (XMCD) of a Bi2212 single-crystal near-optimum doping. The Cu K-edge XMCD signal was measured at ID12 beamline of ESRF with the k-vector of X-ray beam parallel to c-axis, i.e., with the electric field of X-ray beam E//ab, using a 17-T magnetic field parallel to the c-axis of a Bi2212 single crystal. Numerical simulations of the XMCD signal of Bi2212 by multiple scattering theory have shown agreement with the experimental XMCD signal only for the local structure with noncentrosymmetric Bb2b space group of Bi2Sr2CaCu2O8+y. More... »

PAGES

663-670

References to SciGraph publications

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    50 cuprate superconductors
    51 dichroism
    52 doping
    53 edge X
    54 edge XANES
    55 edge XMCD signals
    56 electric field
    57 evidence
    58 experimental XMCD signal
    59 field
    60 group
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    62 lamellar system
    63 large majority
    64 lattice
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    66 local noncentrosymmetric symmetry
    67 local structure
    68 magnetic circular dichroism
    69 magnetic field
    70 majority
    71 multiple scattering theory
    72 near-optimum doping
    73 new compelling results
    74 noncentrosymmetric Bb2b space group
    75 noncentrosymmetric structure
    76 noncentrosymmetric symmetry
    77 numerical simulations
    78 parallel
    79 prototype cuprate superconductor
    80 ray beam E//ab
    81 ray beam parallel
    82 ray magnetic circular dichroism
    83 results
    84 scattering theory
    85 signals
    86 simulations
    87 single crystals
    88 single-crystal near-optimum doping
    89 space group
    90 stack
    91 structure
    92 studied prototype cuprate superconductor
    93 superconductivity
    94 superconductors
    95 symmetry
    96 system
    97 tetragonal CuO2 lattice
    98 theory
    99 unconventional high Tc superconductivity
    100 vector
    101 ySr2 O2 layers
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