Large Magnetocaloric Effect at the Saturation Field of an S=1/2 Antiferromagnetic Heisenberg Chain View Full Text


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Article Info

DATE

2010-01-06

AUTHORS

M. Lang, Y. Tsui, B. Wolf, D. Jaiswal-Nagar, U. Tutsch, A. Honecker, K. Remović-Langer, A. Prokofiev, W. Assmus, G. Donath

ABSTRACT

We report low-temperature magnetization measurements on a copper-containing coordination polymer [Cu(μ-C2O4)(4-aminopyridine)2(H2O)]n. According to these measurements and previous results (Prokofiev et al. in Cryst. Res. Technol. 42, 394, 2007), the material is a very good realization of an S=1/2 antiferromagnetic Heisenberg chain with a small saturation field Bs=4.2 T, which marks the endpoint of a quantum-critical line in the B–T plane. Measurements of the magnetocaloric effect at low temperatures T=0.47 K across the saturation field yields a very large magnetothermal response with a characteristic sign change close to the quantum-critical point. The data are in good agreement with the quantum-critical behavior calculated on the basis of exact diagonalization and quantum Monte Carlo simulations. More... »

PAGES

88-91

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10909-009-0092-8

DOI

http://dx.doi.org/10.1007/s10909-009-0092-8

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https://app.dimensions.ai/details/publication/pub.1031838318


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