Complexation of Donor-Acceptor Substituted Aza-Crowns with Alkali and Alkaline Earth Metal Cations. Charge Transfer and Recoordination in Excited State View Full Text


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Article Info

DATE

2015-12-16

AUTHORS

Valery V. Volchkov, Fedor E. Gostev, Ivan V. Shelaev, Viktor A. Nadtochenko, Svetlana N. Dmitrieva, Sergey P. Gromov, Mikhail V. Alfimov, Mikhail Ya. Melnikov

ABSTRACT

Complexation between two aza-15-crown-5 ethers bearing electron donor and acceptor fragments and alkali and alkaline earth perchlorates has been studied using absorption, steady-state fluorescence and femtosecond transient absorption spectroscopy. The spectral-luminescent parameters, the stability and dissociation constants of the complexes were calculated. The intramolecular charge transfer reaction takes place both in the excited state of the crowns and their complexes 1:1; the latter is subjected to photorecoordination resulting in a weakening or a complete disruption of coordination bond between nitrogen atom and metal cation, disposed within a cavity of the crown. The compounds investigated can be viewed as novel optical molecular sensors for alkali and alkaline-earth metal cations. The photoejection of a metal cation into the bulk was not observed. More... »

PAGES

585-592

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10895-015-1744-5

DOI

http://dx.doi.org/10.1007/s10895-015-1744-5

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1001202870

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/26670689


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191 grid-institutes:grid.465313.6 schema:alternateName Photochemistry Center, Russian Academy of Sciences, 7A-1 Novatorov str., 119421, Moscow, Russia
192 schema:name Chemistry Department, M. V. Lomonosov Moscow State University, 1-3 Leninskie gory, 119991, Moscow, Russia
193 Photochemistry Center, Russian Academy of Sciences, 7A-1 Novatorov str., 119421, Moscow, Russia
194 rdf:type schema:Organization
195 grid-institutes:grid.4886.2 schema:alternateName N. N. Semenov Institute of Chemical Physics, Russian Academy of Sciences, 4 Kosygina str., 119991, Moscow, Russia
196 schema:name Chemistry Department, M. V. Lomonosov Moscow State University, 1-3 Leninskie gory, 119991, Moscow, Russia
197 N. N. Semenov Institute of Chemical Physics, Russian Academy of Sciences, 4 Kosygina str., 119991, Moscow, Russia
198 rdf:type schema:Organization
 




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