Synthesis, Photophysical and Redox Properties of the D–π–A Type Pyrimidine Dyes Bearing the 9-Phenyl-9H-Carbazole Moiety View Full Text


Ontology type: schema:ScholarlyArticle     


Article Info

DATE

2015-05

AUTHORS

Egor V. Verbitskiy, Aleksandr V. Schepochkin, Nadezhda I. Makarova, Igor V. Dorogan, Anatoly V. Metelitsa, Vladimir I. Minkin, Sergey A. Kozyukhin, Victor V. Emets, Vitaly A. Grindberg, Oleg N. Chupakhin, Gennady L. Rusinov, Valery N. Charushin

ABSTRACT

Novel donor-π-acceptor dyes bearing the pyrimidine unit as an electron-withdrawing group have been synthesized by using combination of two processes, based on the microwave-assisted Suzuki cross-coupling reaction and nucleophilic aromatic substitution of hydrogen. Spectral properties of the obtained dyes in six aprotic solvents of various polarities have been studied by ultraviolet-visible and fluorescence spectroscopy. In contrast to the absorption spectra, fluorescence emission spectra displayed a strong dependence from their solvent polarities. The nature of the observed long wavelength maxima has been elucidated by means of quantum chemical calculations. The electrochemical properties of these dyes have been investigated by using cyclic voltammetry, while their photovoltaic performance was evaluated by a device fabrication study. The experimental and calculation data show that all of the dyes can be regarded as potentially good photosensitizers for dye-sensitized solar cells. More... »

PAGES

763-775

References to SciGraph publications

Identifiers

URI

http://scigraph.springernature.com/pub.10.1007/s10895-015-1565-6

DOI

http://dx.doi.org/10.1007/s10895-015-1565-6

DIMENSIONS

https://app.dimensions.ai/details/publication/pub.1018120239

PUBMED

https://www.ncbi.nlm.nih.gov/pubmed/25822191


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